Measurement of radon exhalation rate from building materials: The case of Mashhad-Khorasan Region Iran

Document Type : Original Article

Authors

Department of Physics, Payame Noor University, Tehran, Iran

Abstract

The release of Radon gas from soil, water and building materials in closed environments exposes residents to this radioactive gas. Although humans use building materials as a protective barrier against the natural radiation of the open space, the radionuclide compounds released from some building materials cause an increase in indoor radon concentration. Therefore, measuring the amount of Radon exhalation from building materials is very important for public health.  Although Radon is the most important source of natural radiation and its high concentration level in the closed environments has a significant health risk, the main daughter nuclei of radon, 214Po and 218Po isotopes, have also a high ability to cause lung cancer in humans. Therefore, public attention and concern about the release of radon from building materials used in the indoor environments have increased recently and many efforts have been done to evaluate and control indoor radon concentrations. In this paper, the surface diffusion coefficient of radon from samples of widely used building materials was measured and calculated using the active method in the closed chamber and Sarad-RTM1689 radon meter. The results obtained for the exhalation rate of radon gas for these samples vary from the range of undetectable insignificant values up to 1.95 Bqm-2h-1. The highest surface exhalation rate was observed in granite samples, while the clay brick sample showed a rate lower than the detection threshold (0.05 Bq m-2h-1). From our results it can be suggested to choose more suitable building materials for a safer indoor environment.

Keywords


  1. World Health Organization, WHO Handbook on Indoor Radon: a public health perspective, Geneva, 2009.
  2. International Atomic Energy Agency, Protection of the Public against Exposure Indoors due to Radon and Other Natural Sources of Radiation, Specific Safety Guide No. SSG-32, Vienna, Specific Safety Guide No. SSG-32, 2015.
  3. P. Ujić, I. Čeliković, A. Kandić, I. Vukanac, M. Đurašević, D. Dragosavac, Z. S. Žunić. Internal exposure from building materials exhaling 222Rn and 220Rn as compared to external exposure due to their natural radioactivity content. Appl. Radiat. Isot. 68 (1) (2010) 201-206.
  4. V. Dentoni, S. Da Pelo, M. M. Aghdam, P. Randaccio, A. Loi, N. Careddu, A. Bernardini. Natural radioactivity and radon exhalation rate of sardinian dimension stones. Construction Build. Mater. 247 (2020). 118377.
  5. R. C. Bruno. Sources of indoor radon in houses: A review. J. Air Pollution Control Association 33 (2) (1983) 105-109.
  6. S. Stoulos, M. Manolopoulou, C. Papastefanou. Assessment of natural radiation exposure and radon exhalation from building materials in Greece. J. Environ. Radioactivity 69 (3) (2003) 225-240.
  7. S. Righi, L. Bruzzi. Natural radioactivity and radon exhalation in building materials used in italian dwellings. J. Environ. Radioactivity 88 (2) (2006) 158-170.
  8. N. M. Hassan, T. Ishikawa, M. Hosoda, A. Sorimachi, S. Tokonami, M. Fukushi, S. K. Sahoo. Assessment of the natural radioactivity using two techniques for the measurement of radionuclide concentration in building materials used in Japan. J. Radioanalytical Nucl. Chem. 283 (1) (2010) 15-21.
  9. S. M. Zabihinpour, A. A .Mowlavi, B. Azadegan. The role of natural ventilation on reducing indoor radon concentration. J. Radiat. Safety Measurement 7 (4) (2018) 1-10.
  10. F. Asgharizadeh, M. Ghannadi Maragheh, B. Salimi, E. Sedgh Gouya. Dose rate calculation caused by natural radioactivity in granite samples used as building materials in Iran. J. Radiat. Safety Measurement 3 (2) (2014) 27-33.
  11. N. Zareie, M. R. Rezaie Rayeni Nejad. Estimation of radiation hazards caused by granite in the villages of Dehsiahan, Khanaman and Mani in Rafsanjan city of Kerman province. J. Radiat. Safety Measurement 11 (5) (2023) 25–32.
  12. F. Asgharizadeh, M. Esmailnezhad, P. Pourdeh, F. Moatar, A. Sadigzadeh, E. Sedgh Gouya, P. Nasiri. Measurement and comparison of radioactivity concentration of radon indoor air of buildings faced by granite and carbonate. J. Radiat. Safety Measurement 2 (1) (2013) 11-14.
  13. M. Jafarizadeh, M. Zahedifar, M. Taheri, S. Measurement of radon concentration in some dwellings of Kashan city in Iran. J. Radiat. Safety Measurement 3 (2) (2014) 37-41.
  14. F. Asgharizadeh, M. Ghannadi Maragheh, B. Salimi, E. Sedgh Gouya. Dose rate calculation caused by natural radioactivity in granite samples used as building materials in Iran. J. Radiat. Safety Measurement 3 (2) (2022) 27-30.
  15. M. Pirsaheb, F. Najaf, A. Haghparast, L.Hemati, K. Sharafi, N. The influence of internal wall and floor covering materials and ventilation type on indoor radon and thoron levels in hospitals of Kermanshah, Iran. Iran. Red. Crescent Med. J. 18 (10) (2016) e25292.
  16. A. Soltani, A. Moradi. Microscopic Observations and Natural Radioactivity Hazzard Indices in Granites Used in Dwelling. J. Sustainable. Architecture Urban Design.(1) (2018) 1-22.
  17. A. Abbasi. Calculation of gamma radiation dose rate and radon concentration due to granites used as building materials in Iran. Radiat. Prot. Dosimetry 155 (3) (2013) 335-342.
  18. I. T. Čeliković, G. K. Pantelić, M. Z. Živanović, I. S. Vukanac, J. D. Krneta Nikolić. Radon and thoron exhalation rate measurements from building materials used in Serbia. Nukleonika 65 (2) (2020) 111–114.
  19. T. Tene, C. V. Gomez, G. T. Usca, B. Suquillo, S. Bellucci. Measurement of radon exhalation rate from building materials: The case of highland region of Ecuador. Construction Build. Mater. 293 (2021) 123282.
  20. C. Y. H. Chao, T. C. W. Tung, D. W. T. Chan, J. Burnett. Determination of radon emanation and back diffusion characteristics of building materials in small chamber tests. Build. Environ. 32 (4) (1997) 355-362.
  21. P. Tuccimei, M. Moroni, D. Norcia. Simultaneous determination of 222Rn and 220Rn exhalation rates from building materials used in central italy with accumulation chambers and a continuous solid state alpha detector: influence of particle size, humidity and precursors concentration. Appl. Radiat. Isot. 64 (2) (2006) 254-263.
  22. G. Keller, B. Hoffmann, T. Feigenspan. Radon permeability and radon exhalation of building materials. Sci. Total Environ. 272 (1-3) (2001) 85-89.
  23. L. Zhang, X. Lei, Q. Guo, S. Wang, X. Ma, Z. Shi. Accurate measurement of the radon exhalation rate of building materials using the closed chamber method. J. Radiol. Prot. 32 (3) (2012) 315-323.
  24. K. Kovler, A. Perevalov, V. Steiner, E. Rabkin. Determination of the radon diffusion length in building materials using electrets and activated carbon. Health Phys. 86 (5) (2004) 505–516.
  25. C. E. Andersen. Radon-222 exhalation from Danish building materials: H + H Industri A/S results. Risø National Laboratory, Roskilde, Denmark, 1999.
  26. N. Petropoulos, M. Anagnostakis, S. Simopoulos. Building materials radon exhalation rate: Erricca intercomparison exercise results. Sci. Total Environ. 272 (1-3) (2001) 109-118.
  27. J. Chen, N. M. Rahman, I. A. Atiya. Radon exhalation from building materials for decorative use. J. Environ. Radioactivity 101 (4) (2010) 317-322.
  28. H. Friedmann, C. Nuccetelli, B. Michalik, M. Anagnostakis, G. Xhixha, K. Kovler, G. de With, C. Gascó, W. Schroeyers, R. Trevisi, S. Antropov, A. Tsapalov, C. Kunze, N. P. Petropoulos. Measurement of Norm. Naturally Occurring Radioactive Materials in Construction: Integrating Radiation Protection in Reuse (COST Action Tu1301 NORM4BUILDING). Schroeyers, W. (ed.). Duxford, UK: Woodhead Publishing Limited, (2017) pp. 61-133.
  29. C. Samuelsson, H. Pettersson. Exhalation of 222Rn from porous materials. Radiat. Prot. Dosimetry 7 (1-4) (1984) 95-100.
  30. C. Samuelsson. The closed-can exhalation method for measuring radon. J. Res. Nat. Inst. Stand. Technol. 95 (2) (1990) 167-169.
  31. S. M. Zabihinpour, Z. Khaniki. Designing an effective method for rapid estimation of surface radon emission rate from building materials. Nat. Conf. Technol. Adv. Appl. Phys. (2022).
  32. G. Sarkheil, D. Shirkhani, Y. Azimi, A. Talebi. Identification of natural radon gas emission zones in Mashhad and implementing its pollution reduction system at the site-scale. J. Earth Sci. Kharazmi 7 (2) (2022) 131-119.